双月刊

ISSN 1006-9585

CN 11-3693/P

+高级检索 English
亚洲地区夏季风期间氨气的时空分布特征
DOI:
作者:
作者单位:

中国气象科学研究院

作者简介:

通讯作者:

基金项目:


Temporal and Spatial Distribution Characteristics of Ammonia during the Asian Summer Monsoon
Author:
Affiliation:

Chinese Academy of Meteorological Sciences

Fund Project:

  • 摘要
  • |
  • 图/表
  • |
  • 访问统计
  • |
  • 参考文献
  • |
  • 相似文献
  • |
  • 引证文献
  • |
  • 资源附件
    摘要:

    氨气(NH3)是大气中含量最丰富的碱性气体,是颗粒态NH4+的唯一来源,在二次无机盐生成中起着重要作用。NH3极易与大气中的硝酸(HNO3)和硫酸(H2SO4)发生酸碱中和反应,生成硝酸铵(NH4NO3)和硫酸铵((NH4)2SO4)等二次无机气溶胶,因此,NH3的排放、输送及化学转化过程对全球无机气溶胶的时空分布有重要影响。本文利用ENVISAT卫星搭载的迈克尔逊干涉仪(MIPAS)和Aqua卫星搭载的AIRS探测仪观测到的大气NH3浓度数据,以及全球大气化学-气候模式EMAC模拟的NH3结果,分析了2008-2011年6-9月亚洲地区大气NH3的空间分布特征。结果显示,近地面NH3浓度最高值出现在印度北部,紧邻印度北部的孟加拉湾夏季存在深对流,在印度北部和青藏高原上空出现了NH3的向上输送柱,青藏高原是NH3向上输送的主要通道,NH3虽然寿命短,但在深对流区域可以被输送到上对流层和下平流层(UTLS)。亚洲夏季风反气旋的位置主导着NH3在UTLS区域的空间分布,反气旋内持续存在NH3高浓度中心,NH3高浓度中心位置与反气旋中心位置对应良好,会出现一个或两个NH3高浓度中心,说明反气旋内环流形式的变化对反气旋内NH3分布特征有重要影响。

    Abstract:

    Ammonia (NH3) is the most abundant alkaline gas in the atmosphere and the only source of particulate NH4+, playing an important role in the formation of secondary inorganic salts. NH3 can easily react with nitric acid (HNO3) and sulfuric acid (H2SO4) in the atmosphere to form secondary inorganic aerosols such as ammonium nitrate (NH4NO3) and ammonium sulfate ((NH4)2SO4). Therefore, the emission, transportation, and chemical transformation of NH3 have an important impact on the spatial and temporal distribution of global inorganic aerosols. In this paper, the atmospheric NH3 concentration observed by the Michelson interferometer (MIPAS) on ENVISAT satellite and the AIRS detector on Aqua satellite, as well as simulated by the global atmospheric chemistry climate model EMAC, are used to analyze the spatial distribution characteristics of atmospheric NH3 in East Asia from June to September in 2008-2011. The results show that the highest concentration of NH3 near the surface appears in northern India, and deep convection exists in the Bay of Bengal near northern India in summer. The upward transport column of NH3 appears over northern India and the Qinghai-Tibet Plateau. Although NH3 has a short lifetime, it can be transported to the upper troposphere and lower stratosphere (UTLS) in the deep convection region. During the Asian summer monsoon, the location of the anticyclone dominates the spatial distribution of NH3 in the UTLS. The location of the Asian summer monsoon anticyclone dominates the spatial distribution of NH3 in the UTLS area. The high concentration center of NH3 continues to exist in the anticyclone. The position of the high concentration center of NH3 corresponds well to the position of the center of the anticyclone, and there exist one or two NH3 high concentration centers, indicating that the change of the circulation pattern in the anticyclone has an important influence on the distribution of NH3 in the anticyclone.

    参考文献
    相似文献
    引证文献
引用本文
分享
文章指标
  • 点击次数:
  • 下载次数:
  • HTML阅读次数:
  • 引用次数:
历史
  • 收稿日期:2021-07-14
  • 最后修改日期:2022-03-02
  • 录用日期:2022-05-21
  • 在线发布日期: 2022-05-21
  • 出版日期: