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一个适用于地球系统模式(CAS-ESM)的在线气溶胶与大气化学分量模式(IAP-AACM)的发展与评估
作者:
作者单位:

1.中国科学院大气物理研究所大气边界层物理与大气化学国家重点实验室北京100029;2.中国科学院大学北京100049;3.中国科学院城市环境研究所区域大气环境研究卓越创新中心福建厦门361021;4.中国科学院大气物理研究所国际气候与环境科学中心北京100029;5.中国环境监测总站北京100012;6.纽约州立大学石溪分校纽约11790

作者简介:

王自发,男,1972年出生,博士,研究员,主要从事大气污染输送和沉降、大气化学模式研发、空气质量预报理论与方法研究。E-mail: zifawang@mail.iap.ac.cn

通讯作者:

基金项目:

国家重点研发计划高性能计算专项2016YFB0200800,国家自然科学基金国际(地区)合作与交流项目 41620104008;国家自然科学基金青年科学基金项目 41705108;41605104国家重点研发计划高性能计算专项2016YFB0200800,国家自然科学基金国际(地区)合作与交流项目41620104008,国家自然科学基金青年科学基金项目41705108、41605104


Development and Evaluation of the Online Aerosol and Atmospheric Chemistry Model for the Chinese Academy of Sciences Earth System Model
Author:
Affiliation:

1.State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029;2.University of Chinese Academy of Sciences, Beijing 100049;3.Center for Excellence in Urban Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen, Fujian Province 361021;4.International Center for Climate and Environment Sciences, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029;5.China National Environmental Monitoring Center, Beijing 100012;6.State University of New York at Stony Brook, New York, 11790, USA

Fund Project:

National Major Research High Performance Computing Program of China 2016YFB0200800;Projects of International Cooperation and Exchanges of the National Natural Science Foundation of China 41620104008;National Natural Science Foundation of China Grants ┣41705108;41605104┫Funded by National Major Research High Performance Computing Program of China (Grant 2016YFB0200800), Projects of International Cooperation and Exchanges of the National Natural Science Foundation of China (Grant 41620104008), National Natural Science Foundation of China (Grants 41705108 and 41605104)

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    摘要:

    地球系统模式是研究全球气候与生态环境变化问题的重要工具,气溶胶与大气化学模式负责为其中的大气环流模式提供与气候效应有关的气态化学物质和气溶胶成分。本文在全球嵌套网格空气质量预报模式系统的基础上发展了一个适用于中国科学院地球系统模式(CAS-ESM)耦合计算的气溶胶与大气化学分量模式(IAP-AACM),采用简化的气相化学机制,不仅考虑了人为气溶胶,同时考虑了海盐、沙尘和二甲基硫等自然气溶胶及其前体物的在线排放。评估结果表明,IAP-AACM氧化剂插值计算可靠,采用简化机制和碳键机制(CBM-Z)模拟的差异较小。和观测的对比表明,得益于CAS-ESM的气溶胶双向反馈作用,简化版能够较好地抓住气溶胶及其前体物的空间分布,为IAP-AGCM提供可靠的气溶胶模拟。另外,简化版能大幅提升计算效率,满足CAS-ESM耦合长期积分的需求。为了在全球气候变化的研究中提供更完善的气溶胶模拟,未来考虑在IAP-AACM中增加氮化学和臭氧平流层化学机制。

    Abstract:

    The earth system model (ESM) is an important tool for analyzing global climate and ecological environment changes. The Aerosol and Atmospheric Chemistry Model (AACM) enables the simulation of gases and aerosols associated with the effects of climate change for further processing using the Atmospheric General Circulation Model (AGCM). On the basis of the Global Nested Grid Air Quality Prediction Model System, a simplified version of the AACM of the Institute of Atmospheric Physics (IAP-AACM) suitable for the ESM of the Chinese Academy of Sciences (CAS-ESM) is developed using a simplified gas-phase chemical mechanism. Not only anthropogenic aerosols but also natural aerosols and its precursors (e.g., sea salt, dust, and dimethyl sulfide) are considered. The evaluation showed that the IAP-AACM with simplified gas-phase chemical mechanism can reasonably simulate the spatial distribution of aerosols and precursor gases. The difference between the simplified version and the standard version with CBM-Z mechanism is small. The comparison of the obtained values with the observations shows that the simplified version captured the spatial distribution of aerosols and its precursors well and provided a reliable aerosol simulation for the IAP-AGCM in favor of two-way feedback. Furthermore, the simplified version can significantly improve the calculation efficiency and well satisfy the need for long-range integration of the CAS-ESM. To provide a more comprehensive aerosol simulation in the research on global climate change, the mechanism of nitrogen chemistry and the stratospheric chemistry of ozone will be considered in the IAP-AACM in the future.

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王自发,魏颖,陈学舜,陈焕盛,何卷雄,费可测,李杰,王威,张明华.2020.一个适用于地球系统模式(CAS-ESM)的在线气溶胶与大气化学分量模式(IAP-AACM)的发展与评估[J].气候与环境研究,25(1):1-18. WANG Zifa, WEI Ying, CHEN Xueshun, CHEN Huansheng, HE Juanxiong, FEI Kece, LI Jie, WANG Wei, ZHANG Minghua.2020. Development and Evaluation of the Online Aerosol and Atmospheric Chemistry Model for the Chinese Academy of Sciences Earth System Model[J]. Climatic and Environmental Research (in Chinese],25(1):1-18.

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  • 收稿日期:2019-05-15
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  • 在线发布日期: 2020-03-09
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